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FLOATSUBSCRIPTCl below 115 Okay. Its Br-containing analogue is stable within the room-temperature crystal structure right down to no less than 10 Okay, though the Br compound is on the verge of the same antiferroelectric instability and reveals local displacements of Cu and Br atoms. The I-containing compound is stable in its room-temperature structure according to density-functional calculations. These parameters are chosen in a semi-empirical manner as providing finest settlement with the experimental change couplings in earlier DFT calculations for francisites Rousochatzakis et al. Short-vary AFM order is formed round 50 Okay, but no signatures of lengthy-vary ordering are seen all the way down to 2 Okay. This habits might be rationalized on the microscopic degree by the spin lattice comprising strong non-frustrated one-dimensional (1D) units with solely weak and annoyed couplings between them. FLOATSUBSCRIPTCl, but its magnetic habits is remarkably totally different. This conduct is rationalized microscopically by way of a non-frustrated 1D spin ladder (tube) with comparatively weak and pissed off couplings between the 1D items. ARG antiferromagnets could be orders of magnitude decrease than the energy scale of alternate couplings Janson et al. FLOATSUBSCRIPT tetrahedra. A lot of the trade couplings happen between nearest neighbors, however dissimilar interactions on the edges of these tetrahedra largely cut back the frustration and render the spin lattice quasi-1D.

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